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• W2913449065 abstract "An unprecedented conversion of terminal alkynes into N-sulfonimidamides (amidines) is reported by a silver-catalyzed, one-pot, four-component reaction with TMSN3, sodium sulfinate, and sulfonyl azide. The reaction scope includes both aromatic and aliphatic alkynes. A possible cascade reaction mechanism, consisting of alkyne hydroazidation, sulfonyl radical addition, 1,3-dipolar cycloaddition by TMSN3, and retro-1,3-dipolar cycloaddition, is proposed. TMSN3 is found to play an essential role in each step of the reaction." @default.
• W2913449065 created "2019-02-21" @default.
• W2913449065 creator A5007550988 @default.
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• W2913449065 date "2019-01-22" @default.
• W2913449065 modified "2023-10-16" @default.
• W2913449065 title "Direct Transformation of Terminal Alkynes into Amidines by a Silver-Catalyzed Four-Component Reaction" @default.
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• W2913449065 doi "https://doi.org/10.1021/jacs.8b11039" @default.
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