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• W2914053399 endingPage "1808043" @default.
• W2914053399 startingPage "1808043" @default.
• W2914053399 abstract "The development of robust and efficient trifunctional catalysts for oxygen reduction reaction (ORR), oxygen evolution reaction (OER), and hydrogen reaction (HER) is central to regenerative metal-air batteries and overall water splitting. It is still a big challenge to achieve an efficient integration of three functions in one freestanding electrode. Herein, a facile and upscalable strategy is demonstrated, to construct cobalt nanoparticle-encapsulated 3D conductive films (Co/CNFs), which were induced by in situ solid diffusion from bulk cobalt metal. Under high-temperature, volatile cobalt species from bulk cobalt foil are trapped by the contacted nitrogen-rich carbons, followed by catalytic growth of interconnected carbon tubes, forming the 3D structured film. This resulting film can be directly preformed as self-supporting and binder-free electrode, which simultaneously facilitates the ORR, OER, and HER with excellent activities and superior stability. Furthermore, such all-in-one film also exhibits remarkable performance for Zn-air batteries and overall water splitting, demonstrating its feasibility for practical applications." @default.
• W2914053399 created "2019-02-21" @default.
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• W2914053399 date "2019-02-05" @default.
• W2914053399 modified "2023-10-14" @default.
• W2914053399 title "Trifunctional Self‐Supporting Cobalt‐Embedded Carbon Nanotube Films for ORR, OER, and HER Triggered by Solid Diffusion from Bulk Metal" @default.
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• W2914053399 doi "https://doi.org/10.1002/adma.201808043" @default.
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