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- W2914104451 abstract "To effectively separate lanthanides (Ln(III)) from actinides (An(III)), symmetrical 2,2′-bipyridyl (Bpy), 1,10-phenanthroline (Phen), and unsymmetrical N-methyl-N-tolyl-1,10-phenanthroline-2-carboxamide (MeTol-PTA) were investigated. According to the crystal structures and EXAFS experiments, the decreasing ionic radius from light to heavy Ln led to decreases in the Ln–N (Bpy) and Ln–N (Phen) distances, while log β simply increased due to the electrostatic interaction and the order of Ln–O (MeTol-PTA) < Ln–N (Bpy, Phen) < Ln–N (MeTol-PTA) was obtained. This indicated that the bulky phenanthroline moiety of MeTol-PTA may not allow N (MeTol-PTA) to come close to Ln. Consequently, the log β of MeTol-PTA exhibited a local maximum (around Nd)." @default.
- W2914104451 created "2019-02-21" @default.
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- W2914104451 date "2018-11-10" @default.
- W2914104451 modified "2023-09-24" @default.
- W2914104451 title "Relationship Between Structure and Coordination Strength of <i>N</i> and <i>N,O</i>-Hybrid Donor Ligands with Trivalent Lanthanides" @default.
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- W2914104451 doi "https://doi.org/10.1080/07366299.2018.1532137" @default.
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