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• W2914570404 abstract "This work presents a dense ceramic-carbonate membrane as a new kind of reactor, where CO oxidation and CO2 permeation processes are subsequently produced. This kind of membrane reactors may be applied for hydrogen enrichment of syngas mixtures. In here, a composite (doped-ceria and perovskite) was synthesized, sintered, and infiltrated with molten carbonates, showing that the reactor is able to perform both processes: the CO oxidation at the membrane reactor surface and subsequent CO2 permeation through the molten carbonate phase. Moreover, results evidenced that perovskite phase importantly improves the oxygen permeation from the sweep to feed side (inverse permeation), enhancing CO oxidation and CO32– formation without releasing oxygen on the feed side. When oxidation-permeation test was evaluated on a synthetic syngas mixture (H2 + CO), it was observed that this membrane reactor has an important selectivity for CO oxidation, over hydrogen oxidation, confirming the possible use of this kind of membrane reactors for hydrogen enrichment in different applications." @default.
• W2914570404 created "2019-02-21" @default.
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• W2914570404 date "2019-01-30" @default.
• W2914570404 modified "2023-10-06" @default.
• W2914570404 title "Development of New Bifunctional Dense Ceramic-Carbonate Membrane Reactors for Gas Mixtures Separation, through CO Oxidation and Subsequent CO₂ Permeation" @default.
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• W2914570404 doi "https://doi.org/10.1021/acsaem.8b01947" @default.
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