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• W2914891731 abstract "Construction of N-substituted pyrrolidones from biomass-derived levulinic acid (LA) via reductive amination is a highly attractive route for biomass valorization. However, realizing this transformation using H2 as the hydrogen source under mild conditions is still very challenging. Herein, we designed porous TiO2 nanosheets-supported Pt nanoparticles (Pt/P-TiO2) as the heterogeneous catalyst. The prepared Pt/P-TiO2 was highly efficient for reductive amination of LA to produce various N-substituted pyrrolidones (34 examples) at ambient temperature and H2 pressure. Meanwhile, Pt/P-TiO2 showed good applicability for reductive amination of levulinic esters, 4-acetylbutyric acid, 2-acetylbenzoic acid, and 2-carboxybenzaldehyde. Systematic studies indicated that the strong acidity of P-TiO2 and the lower electron density of the Pt sites as well as the porous structure resulted in the excellent activity of Pt/P-TiO2." @default.
• W2914891731 created "2019-02-21" @default.
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• W2914891731 date "2019-02-10" @default.
• W2914891731 modified "2023-10-16" @default.
• W2914891731 title "Ambient Reductive Amination of Levulinic Acid to Pyrrolidones over Pt Nanocatalysts on Porous TiO₂ Nanosheets" @default.
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• W2914891731 doi "https://doi.org/10.1021/jacs.8b13024" @default.
• W2914891731 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30739440" @default.
• W2914891731 hasPublicationYear "2019" @default.
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