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- W2915049069 abstract "Low energy ion beam deposition of mass-selected fullerene ions was used to generate thin films of non-IPR fullerenes, C2n (2n = 48–58 and 52–68) on graphite under UHV. These were probed by mass-resolved thermal desorption spectroscopy. We observe the emission of dimers in addition to dominant monomer desorption for 2n = 58–68, while for 2n = 48–56 no dimer desorption was detected. Dimer signals were typically at <1% level compared to the monomers. The desorption temperature ranges of these dimer species were higher and much narrower than for the corresponding monomers. Building also on theoretical considerations, we came to the conclusion that coalescence reactions between the fullerenes must take place below 1000 K and that fullerenes with more than three pairs of adjacent pentagons cross-link too strongly to allow the desorption of dimers." @default.
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- W2915049069 date "2019-02-11" @default.
- W2915049069 modified "2023-09-23" @default.
- W2915049069 title "Desorption of Fullerene Dimers upon Heating Non-IPR Fullerene Films on HOPG" @default.
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- W2915049069 doi "https://doi.org/10.1021/acs.jpcc.8b12113" @default.
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