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- W2915261453 abstract "Enantioselective synthesis of thiazole‐containing α‐perfluoroalkylated cyclic amines was elaborated. Organocatalytic Strecker reaction with 5–7 membered cyclic ketimines was used as a key step of sequence. The prepared chiral amino nitriles bearing CF 3 ‐ or C 2 F 5 ‐group in the alpha position were transformed into the corresponding chiral thioamides by the reaction with hydrogen sulfide. Subsequent reaction with alpha bromo‐ or chloro‐substituted carbonyls allowed obtaining perfluoroalkylated analogues of natural thiazole‐containing cyclic amines in high isolated yield and up to > 99 % ee ." @default.
- W2915261453 created "2019-03-02" @default.
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- W2915261453 date "2019-02-21" @default.
- W2915261453 modified "2023-09-25" @default.
- W2915261453 title "Enantioselective Synthesis of Thiazole-Derived α-Perfluoroalkylated 5-7-Membered Amines" @default.
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- W2915261453 doi "https://doi.org/10.1002/ejoc.201801845" @default.
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