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- W2915676848 abstract "A rate equation for carbon monoxide consumption showing first order in CO and 0.5 order in hydrogen indicates the rate controlling step involves dissociated hydrogen. The inhibition of the rate with carbon dioxide is also shown. Examination of the hydrocarbon distributions indicates a see-saw effect with the C{sub 4}s representing the fulcrum and methane and C{sub 5}{sup +} the end points. The shift in the distributions tends to be towards the C{sub 5}{sup +} for high pressures and long residence times. This distribution can be shifted by incorporating Ti into the catalysts, but the optimum amount of Ti needs to be determined. The sol gel method of preparing the catalysts tends to produce a less active catalyst than by precipitation of a zirconyl salt. The most active catalyst contained approximately 2% Th/ZrO{sub 2}" @default.
- W2915676848 created "2019-03-02" @default.
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- W2915676848 date "1992-07-27" @default.
- W2915676848 modified "2023-09-27" @default.
- W2915676848 title "Catalyst and process development for synthesis gas conversion to isobutylene. Quarterly report, April 1, 1992--June 30, 1992" @default.
- W2915676848 doi "https://doi.org/10.2172/10123778" @default.
- W2915676848 hasPublicationYear "1992" @default.
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