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• W2915960488 abstract "Ultrafine and highly dispersed PdCu nanoalloys anchored on porous carbon were synthesized by a facile NaBH4 reduction method in a ionic liquid (IL)/water solution system. During the synthesis, the IL solvent can act not only as a stabilizer to slow down the particle growth and prevent the agglomeration, but also as a functional agent to improve the hydrophilicity and sorption property of carbon support due to the functional groups. The resulting PdCu/porous carbon (PdCu/PC) exhibits a remarkable activity for ethanol oxidation in alkaline solution (ethanol oxidation specific activity of 6.54 mA cm−2, only 2.14 mA cm−2 for commercial Pd/C), high poison tolerance (if/ib = 1.09), and excellent catalytic stability (only a loss of 4.3% of the initial ethanol oxidation reaction activity after 100 cycles). The superior performance of PdCu/PC can be ascribed to the abundant active reaction sites of porous carbon, uniform and good dispersion of PdCu nanoaolloys, as well as the strong metal-support interaction. This work is anticipated to be useful for the development of low-cost and highly active catalysts for fuel cells." @default.
• W2915960488 created "2019-03-02" @default.
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• W2915960488 date "2019-04-01" @default.
• W2915960488 modified "2023-09-25" @default.
• W2915960488 title "PdCu nanoalloys deposited on porous carbon as a highly efficient catalyst for ethanol oxidation" @default.
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• W2915960488 doi "https://doi.org/10.1016/j.matchemphys.2019.02.075" @default.
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