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- W2916810965 abstract "Two novel POM‐based metal‐organic frameworks, [Ag 7 (L 1 ) 2 · (µ 2 ‐OH) 4 ][H 3 VW 12 O 40 ] ( 1 ) and [Ag 8 (L 2 ) 4 ][VW 12 O 40 ] · 4H 2 O ( 2 ) have been isolated by altering the isomeric organic ligands {5‐[ n ‐(1,2,4‐triazol‐4‐yl)phenyl]‐1 H ‐tetrazole: n = 3 (HL 1 ); n = 4 (HL 2 )} under hydrothermal conditions. Due to L 1 acts as a V‐shaped linker, compound 1 displays a 3D MOF with three types of metallocycles, in which the Keggin polyanions locat in the largest metallocycle (the size of void ca. 13.31 Å × 13.53 Å). However, when the ligand is replaced by straight ligand L 2 , compound 2 with a different structure is obtained. Although compound 2 is also a 3D MOF, the types of metallocycle are reduced to one. The Keggin polyanions are seated in the only metallocycle (the size of void ca. 13.6 Å × 13.7 Å). In addition, the adsorption behaviors of the title compounds for organic dyes were investigated in detail. In particular, compound 1 could selectively separate MB + from the mixture of MB + /RhB + and MB + /MO – within 5 min, which can be used as a chromatography column for dyes removal." @default.
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- W2916810965 date "2019-03-03" @default.
- W2916810965 modified "2023-10-17" @default.
- W2916810965 title "Metallocycle‐Supported POM‐Based Metal‐Organic Frameworks Assembled from Isomeric N‐Rich Ligands: Structures and Selective Adsorption and Separation of Cationic Dyes" @default.
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- W2916810965 doi "https://doi.org/10.1002/ejic.201900086" @default.
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