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• W2917302352 abstract "Abstract Uranium is widely used in the nuclear industry and it is well known that uranium hydride, UH 3 , forms when uranium is exposed to air. The associated volume change during this transition can cause the surface region to crack, compromising structural integrity. Here, hydriding regions beneath hydride surface craters are studied by secondary ion mass spectroscopy (SIMS) and X-ray photoelectron spectroscopy (XPS). Our results indicate that strain transition regions exist, which are induced by hydrogen with a certain thickness between hydride craters and the uranium bulk. The SIMS and XPS results suggest that hydrogen exists covalently with uranium and oxygen in these transition regions. A micro-scale induction period model based on the transition region and previous hydriding models is developed. Within the so-called micro-scale induction period, hydrogen diffuses and accumulates at particular sites before reaching the critical concentration required to form stoichiometric UH 3 in the transition regions." @default.
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• W2917302352 date "2019-02-26" @default.
• W2917302352 modified "2023-10-16" @default.
• W2917302352 title "Mechanism of surface uranium hydride formation during corrosion of uranium" @default.
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• W2917302352 doi "https://doi.org/10.1038/s41529-019-0073-6" @default.
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