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- W2920805952 abstract "A quantum-kinetic picture of Shockley-Read-Hall-type (SRH) defect-mediated recombination is derived within the nonequilibrium Green's function formalism for an optoelectronic device with selectively contacted, current-carrying extended states and a localized deep defect state in the energy gap. The theory is first tested for recombination from bulk band states and then implemented for defective bipolar homo- and heterojunction thin-film devices with realistic spatial variation of the band edge profile. While the quantum-kinetic treatment reproduces the semiclassical characteristics for a bulk absorber in flat-band and quasiequilibrium conditions, for which the conventional SRH picture is valid, it reveals nonclassical features such as recombination enhancement by tunneling into field-induced subgap states in the presence of large fields, or the complex recombination current flow at heterointerfaces. Being fully compatible with the rigorous treatment of electron-photon and electron-phonon scattering in the nonequilibrium Green's function (NEGF) formalism, the approach enables a consistent inclusion of defect-mediated nonradiative recombination in comprehensive NEGF simulations of nanostructure-based quantum optoelectronic devices such as quantum well lasers, LEDs and solar cells." @default.
- W2920805952 created "2019-03-22" @default.
- W2920805952 creator A5082397926 @default.
- W2920805952 date "2019-03-18" @default.
- W2920805952 modified "2023-09-26" @default.
- W2920805952 title "Nonequilibrium Green's function picture of nonradiative recombination of the Shockley-Read-Hall type" @default.
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- W2920805952 doi "https://doi.org/10.1103/physrevb.99.125302" @default.
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