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- W2921016721 abstract "Summary 90Sr2+ remediation from acidic nuclear waste solution and contaminated seawater attracts great public attention but is very challenging because the removal performance toward soft Sr2+ by traditional oxidic ion-exchange materials are greatly affected by hard cations including H+, Na+, and Ca2+. We report a layered oxidic coordination polymer [(CH3)2NH2][ZrCH2(PO3)2F] (SZ-4) showing a notable advance over existing ion-exchange materials in 90Sr removal efficiencies with elevated distribution coefficients and record-high uptake capacities under acidic conditions. Moreover, the removal of Sr2+ is not significantly affected by the presence of a large excess of hard cations, leading to the successful cleanup of 90Sr-contaminated seawater samples. Such superior capabilities are directly visualized by well-refined single-crystal structures during in situ Sr2+ sorption process, revealing a distinctive two-step intercalation mechanism and a unique soft cation uptake selectivity achieved through collaborative coordination by the host layer and the interlayer dimethylamine (DMA) as a soft N-donor ligand." @default.
- W2921016721 created "2019-03-22" @default.
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- W2921016721 date "2019-04-01" @default.
- W2921016721 modified "2023-10-15" @default.
- W2921016721 title "Distinctive Two-Step Intercalation of Sr2+ into a Coordination Polymer with Record High 90Sr Uptake Capabilities" @default.
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- W2921016721 doi "https://doi.org/10.1016/j.chempr.2019.02.011" @default.
- W2921016721 hasPublicationYear "2019" @default.
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