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• W2921140517 abstract "ABSTRACT 2,5‐Diketopiperazines (DKPs) are the smallest cyclic dipeptides found in nature with various attractive properties. In this study, we have demonstrated the successful modification of proline‐based DKPs using anionic ring‐opening polymerization (AROP) as a direct approach. Four different proline‐based DKPs with various side chains and increasing steric hindrance were used as initiating species for the polymerization of 1,2‐epoxybutane or ethoxyethyl glycidyl ether in the presence of t‐BuP 4 phosphazene base. The addition of a Lewis acid, tri‐isobutyl aluminum, to the reaction mixture strongly decreased the occurrence of side reactions. Impact of the DKP side‐chain functionalities on molar mass control and dispersity was successfully evidenced. © 2019 Wiley Periodicals, Inc. J. Polym. Sci., Part A: Polym. Chem. 2019 , 57 , 1008–1016" @default.
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• W2921140517 date "2019-03-15" @default.
• W2921140517 modified "2023-10-17" @default.
• W2921140517 title "Modification of proline‐based 2,5‐diketopiperazines by anionic ring‐opening polymerization" @default.
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• W2921140517 doi "https://doi.org/10.1002/pola.29356" @default.
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