Matches in SemOpenAlex for { <https://semopenalex.org/work/W2921547560> ?p ?o ?g. }
- W2921547560 endingPage "91" @default.
- W2921547560 startingPage "84" @default.
- W2921547560 abstract "Developing an efficient adsorbent for selective separation and capture of CO2 from CO2/N2 mixture is an important and challenging issue for mitigating global warming. In this study, we posited that high CO2/N2 selectivity could be obtained by impregnating polyethyleneimine (PEI) within the pores of NU-1000, a zirconium-based metal-organic framework (MOF), since it has a high surface area (∼2320 m2/g) and free and exposed OH groups but does not have unsaturated metal sites possibly having strong interactions with N2 molecules. A series of PEI-impregnated NU-1000 (PEI(x)@NU-1000) materials with varied PEI loadings have been successfully prepared. As reasoned, PEI(50)@NU-1000 showed the highest CO2/N2 selectivity among the PEI-loaded adsorbents in the literature under similar conditions. Remarkably, it exhibited extremely high CO2/N2 selectivities (∼8000) at low pressures and a very high CO2/N2 selectivity (661) at a typical pressure of flue gas (1 bar). Furthermore, PEI(50)@NU-1000 could efficiently separate CO2/N2 mixture under a dynamic flow condition and maintained its CO2 uptakes during three consecutive adsorption and desorption." @default.
- W2921547560 created "2019-03-22" @default.
- W2921547560 creator A5003164811 @default.
- W2921547560 creator A5007705659 @default.
- W2921547560 creator A5016518987 @default.
- W2921547560 creator A5023535365 @default.
- W2921547560 creator A5051506761 @default.
- W2921547560 creator A5065050090 @default.
- W2921547560 creator A5082403624 @default.
- W2921547560 date "2019-06-01" @default.
- W2921547560 modified "2023-10-18" @default.
- W2921547560 title "Extraordinarily selective adsorption of CO2 over N2 in a polyethyleneimine-impregnated NU-1000 material" @default.
- W2921547560 cites W1963643295 @default.
- W2921547560 cites W1965437736 @default.
- W2921547560 cites W1987736265 @default.
- W2921547560 cites W1999937609 @default.
- W2921547560 cites W2002039699 @default.
- W2921547560 cites W2010621173 @default.
- W2921547560 cites W2016159385 @default.
- W2921547560 cites W2019293828 @default.
- W2921547560 cites W2022167379 @default.
- W2921547560 cites W2025831662 @default.
- W2921547560 cites W2026972799 @default.
- W2921547560 cites W2031367372 @default.
- W2921547560 cites W2040123693 @default.
- W2921547560 cites W2050343674 @default.
- W2921547560 cites W2053164863 @default.
- W2921547560 cites W2056127514 @default.
- W2921547560 cites W2056747681 @default.
- W2921547560 cites W2059277244 @default.
- W2921547560 cites W2059420540 @default.
- W2921547560 cites W2078913711 @default.
- W2921547560 cites W2093396192 @default.
- W2921547560 cites W2094774149 @default.
- W2921547560 cites W2108623890 @default.
- W2921547560 cites W2121022470 @default.
- W2921547560 cites W2125053394 @default.
- W2921547560 cites W2130360607 @default.
- W2921547560 cites W2152291440 @default.
- W2921547560 cites W2168175046 @default.
- W2921547560 cites W2217138787 @default.
- W2921547560 cites W2257853348 @default.
- W2921547560 cites W2315918039 @default.
- W2921547560 cites W2322571666 @default.
- W2921547560 cites W2510984897 @default.
- W2921547560 cites W2511869034 @default.
- W2921547560 cites W2512327425 @default.
- W2921547560 cites W2514977749 @default.
- W2921547560 cites W2523510937 @default.
- W2921547560 cites W2565783546 @default.
- W2921547560 cites W2607066018 @default.
- W2921547560 cites W2735677792 @default.
- W2921547560 cites W2740425792 @default.
- W2921547560 cites W2753865815 @default.
- W2921547560 cites W2770855437 @default.
- W2921547560 cites W2789308049 @default.
- W2921547560 cites W2884166932 @default.
- W2921547560 cites W2886775537 @default.
- W2921547560 cites W620075937 @default.
- W2921547560 doi "https://doi.org/10.1016/j.micromeso.2019.03.001" @default.
- W2921547560 hasPublicationYear "2019" @default.
- W2921547560 type Work @default.
- W2921547560 sameAs 2921547560 @default.
- W2921547560 citedByCount "30" @default.
- W2921547560 countsByYear W29215475602019 @default.
- W2921547560 countsByYear W29215475602020 @default.
- W2921547560 countsByYear W29215475602021 @default.
- W2921547560 countsByYear W29215475602022 @default.
- W2921547560 countsByYear W29215475602023 @default.
- W2921547560 crossrefType "journal-article" @default.
- W2921547560 hasAuthorship W2921547560A5003164811 @default.
- W2921547560 hasAuthorship W2921547560A5007705659 @default.
- W2921547560 hasAuthorship W2921547560A5016518987 @default.
- W2921547560 hasAuthorship W2921547560A5023535365 @default.
- W2921547560 hasAuthorship W2921547560A5051506761 @default.
- W2921547560 hasAuthorship W2921547560A5065050090 @default.
- W2921547560 hasAuthorship W2921547560A5082403624 @default.
- W2921547560 hasConcept C111368507 @default.
- W2921547560 hasConcept C118792377 @default.
- W2921547560 hasConcept C127313418 @default.
- W2921547560 hasConcept C127413603 @default.
- W2921547560 hasConcept C150394285 @default.
- W2921547560 hasConcept C161790260 @default.
- W2921547560 hasConcept C162711632 @default.
- W2921547560 hasConcept C167206829 @default.
- W2921547560 hasConcept C178790620 @default.
- W2921547560 hasConcept C179104552 @default.
- W2921547560 hasConcept C185592680 @default.
- W2921547560 hasConcept C188721877 @default.
- W2921547560 hasConcept C2777895876 @default.
- W2921547560 hasConcept C42360764 @default.
- W2921547560 hasConcept C534791751 @default.
- W2921547560 hasConcept C544153396 @default.
- W2921547560 hasConceptScore W2921547560C111368507 @default.
- W2921547560 hasConceptScore W2921547560C118792377 @default.
- W2921547560 hasConceptScore W2921547560C127313418 @default.
- W2921547560 hasConceptScore W2921547560C127413603 @default.
- W2921547560 hasConceptScore W2921547560C150394285 @default.