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- W2921578627 abstract "Most of the searches for Kitaev materials deal with $4d/5d$ magnets with spin-orbit-coupled ${J=1/2}$ local moments such as iridates and $alpha$-RuCl$_3$. Here we propose a new Kitaev material candidate YbCl$_3$. We perform thermodynamic, $ac$ susceptibility and angle-dependent magnetic torque measurements on YbCl$_3$ single crystal. We find that the Yb$^{3+}$ ion exhibits a Kramers doublet ground state that gives rise to an effective spin ${J_{text{eff}}=1/2}$ local moment with likely strong anisotropic exchange interactions. The compound exhibits short-range magnetic ordering at around 1.20 K followed by long-range ordering at 0.60 K. These orderings can be suppressed by in-plane and out-of-plane magnetic fields, resulting in a quantum critical point at around 6 and 10 T, respectively. Furthermore, the non-monotonic decrease of Neel temperature under out-of-plane magnetic fields and the 99.8% of ground state entropy release across the short range ordering, strongly suggest that YbCl$_3$ is more two-dimensional than $alpha$-RuCl$_3$ and thus a closer realization of a Kitaev system." @default.
- W2921578627 created "2019-03-22" @default.
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- W2921578627 date "2019-03-08" @default.
- W2921578627 modified "2023-09-24" @default.
- W2921578627 title "a rare-earth Kitaev material candidate YbCl$_3$" @default.
- W2921578627 hasPublicationYear "2019" @default.
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