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• W2922259871 endingPage "245707" @default.
• W2922259871 startingPage "245707" @default.
• W2922259871 abstract "The transport of water through carbon nanotubes (CNTs) is now of great importance in bionanotechnology and of considerable interest for potential nanofluidic applications. In this paper, we show by molecular dynamics simulations that the permeation of single-file water molecules through a CNT can be significantly improved by means of tuning the direction of pressure difference, i.e. introducing an additional lateral pressure to the longitudinal one. The water flow exhibits an interesting maximum behavior with the change of lateral pressure, deciphered by the breakdown of single-file water chain inside the CNT. The translocation time decreases monotonously with the increase of lateral pressure and exhibits a clear bifurcation due to the longitudinal pressure, corresponding to the flow enhancement. Therefore, the lateral pressure will increase the difficulty for water entering, while promotes the water conduction inside the CNT, whose competition ultimately leads to the flow maximum behaviors. Along with the water reducing inside the CNT, the CNT switches between the filling and empty states with the unique distributions of water dipole orientation, density and H-bond number. Our results indicate that tuning the direction of pressure difference should be a significant new strategy for enhancing the water permeability, where the key lies in the breakdown of single-file water chain and are thus insightful for future studies." @default.
• W2922259871 created "2019-03-22" @default.
• W2922259871 creator A5016855897 @default.
• W2922259871 creator A5036485299 @default.
• W2922259871 creator A5066078068 @default.
• W2922259871 date "2019-04-01" @default.
• W2922259871 modified "2023-10-16" @default.
• W2922259871 title "Enhanced water transport through a carbon nanotube controlled by the lateral pressure" @default.
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• W2922259871 doi "https://doi.org/10.1088/1361-6528/ab0cd7" @default.
• W2922259871 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/30836337" @default.
• W2922259871 hasPublicationYear "2019" @default.
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