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- W2922383963 abstract "Herein, novel photoactive materials, MOF-derived porous hollow carbon [email protected] multi-shelled dodecahedral cages ([email protected] MSDCs)， were synthesized via continuous chemical etching, sulfurization, cation-exchange and calcination strategies. Due to the synergistic effect between the porous shells and the carbon-layer coating， [email protected] MSDCs displayed superior photoelectrochemical (PEC) performance. The synthesized [email protected] MSDCs were assembled onto TiO2 modified ITO electrodes to form a type-II heterostructures. Then, Au nanoparticles (NPs) were deposited on the surface of ITO/TiO2/[email protected] MSDCs. Benefiting from the unique structure and performance merits of photoactive materials, a label-free PEC sensing platform based on ITO/TiO2/[email protected] MSDCs/Au was successfully constructed for CEA detection. Under optimal conditions, the PEC biosensor exhibited a wide linear range (0.00005–500 ng mL−1) and low detection limit (2.28 fg mL−1). The proposed PEC biosensor also showed good stability, specificity, reproducibility and acceptability in human serum. The prepared [email protected] MSDCs would be a promising photoactive material for PEC biosensors. Most importantly, this work opens up new horizons for the application of MOFs-derived hollow carbon materials in sensing." @default.
- W2922383963 created "2019-03-22" @default.
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- W2922383963 date "2019-05-01" @default.
- W2922383963 modified "2023-10-12" @default.
- W2922383963 title "Porous hollow carbon nanobubbles@ZnCdS multi-shelled dodecahedral cages with enhanced visible-light harvesting for ultrasensitive photoelectrochemical biosensors" @default.
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- W2922383963 doi "https://doi.org/10.1016/j.bios.2019.03.028" @default.
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