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• W2922473565 abstract "Abstract To assess the mechanism and milder conditions for amines to imines, UiO-66-NH2 was chosen as an efficient photocatalyst for the transformation under light irradiation. A series of experiments for the catching of the active species were performed, and it was proved that holes (h+) and superoxide radicals ( O2−) were involved when the reaction was performed under air. The reaction also occurred because of the presence of nitrogen-centered radical cations and carbon-centered radicals, which were induced by photogenerated hole (h+) with considerable conversion and selectivity under anaerobic conditions. Our experiments revealed that the catalyst can be recycled for four times." @default.
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• W2922473565 date "2019-05-01" @default.
• W2922473565 modified "2023-10-16" @default.
• W2922473565 title "Atmospherical oxidative coupling of amines by UiO-66-NH2 photocatalysis under milder reaction conditions" @default.
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• W2922473565 doi "https://doi.org/10.1016/j.catcom.2019.03.011" @default.
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