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• W2924707551 abstract "Abstract Two‐stage [2π+2σ+2σ]‐cycloaddition of quadricyclane ( 2 ) with 2,3‐dicyano‐1,4‐benzoquinone ( 1 ) with a huge difference in the activity of two reaction centers has been studied. In the first stage (kinetic control), the cycloaddition of 2 takes place on the activated С 2 =С 3 bond of 1 to form the monoadduct 3 , and in the second stage the cycloaddition of 2 on the С 5 =С 6 bond of the monoadduct 3 occurs by 6 orders of magnitude lower with the formation of bisadduct 4 . The structures of adducts 3 and 4 have been proved by NMR data and the X‐Ray method, respectively. The kinetics of the first and second stages, the enthalpy of dissolution of 1 in the π‐donor solvents, and the enthalpy of the reaction 1+2→3 have been measured." @default.
• W2924707551 created "2019-04-01" @default.
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• W2924707551 date "2019-03-22" @default.
• W2924707551 modified "2023-10-14" @default.
• W2924707551 title "Kinetics and thermochemistry of the [2π+2σ+2σ]‐cycloaddition of quadricyclane with 2,3‐dicyano‐1,4‐benzoquinone" @default.
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• W2924707551 doi "https://doi.org/10.1002/kin.21264" @default.
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