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- W2925230356 abstract "Stimulation with ultrafast light pulses can realize and manipulate states of matter with emergent structural, electronic and magnetic phenomena. However, these non-equilibrium phases are often transient and the challenge is to stabilize them as persistent states. Here, we show that atomic-scale PbTiO3/SrTiO3 superlattices, counterpoising strain and polarization states in alternate layers, are converted by sub-picosecond optical pulses to a supercrystal phase. This phase persists indefinitely under ambient conditions, has not been created via equilibrium routes, and can be erased by heating. X-ray scattering and microscopy show this unusual phase consists of a coherent three-dimensional structure with polar, strain and charge-ordering periodicities of up to 30 nm. By adjusting only dielectric properties, the phase-field model describes this emergent phase as a photo-induced charge-stabilized supercrystal formed from a two-phase equilibrium state. Our results demonstrate opportunities for light-activated pathways to thermally inaccessible and emergent metastable states." @default.
- W2925230356 created "2019-04-01" @default.
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- W2925230356 date "2019-03-18" @default.
- W2925230356 modified "2023-10-16" @default.
- W2925230356 title "Optical creation of a supercrystal with three-dimensional nanoscale periodicity" @default.
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- W2925230356 doi "https://doi.org/10.1038/s41563-019-0311-x" @default.
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