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- W2933240131 abstract "The first asymmetric propargylic radical cyanation was realized through a dual photoredox and copper catalysis. An organic photocatalyst serves to both generate propargyl radicals and oxidize Cu(I) species to Cu(II) species. A chiral Cu complex functions as an efficient organometallic catalyst to resemble the propargyl radical and cyanide in an enantio-controlled manner. Thus, a diverse range of optically active propargyl cyanides were produced with high reaction efficiency and enantioselectivities (28 examples, 57-97% yields and 83-98% ee). Moreover, mechanistic investigations including experiments and density functional theory calculations were performed to illustrate on the reaction pathway and stereochemical results." @default.
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- W2933240131 date "2019-03-31" @default.
- W2933240131 modified "2023-10-17" @default.
- W2933240131 title "Asymmetric Propargylic Radical Cyanation Enabled by Dual Organophotoredox and Copper Catalysis" @default.
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- W2933240131 doi "https://doi.org/10.1021/jacs.9b02338" @default.
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