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• W2933321857 abstract "Abstract The development of high-performance electrocatalysts holds the decisive key to the electrochemical CO2 reduction toward value-added products. Formic acid or formate is a desirable reduction product, but its selective production is often challenging. Tin based-materials have attracted great attention for formate production, and yet their performances are far from satisfactory. In this study, we reported the preparation of SnO2 nanoclusters from the controlled self-polymerization of dopamine together with SnO32−, followed by the mild-temperature calcination. The final product consisted of large primary particles that were further made of small secondary SnO2 nanocrystals. When evaluated as the electrocatalyst for CO2 reduction in 0.5 M NaHCO3, our material exhibited impressive activity, selectivity and stability for the selective CO2 reduction to formate. A peak formate Faradaic efficiency of ∼73% and large partial current density of 16.3 mA/cm2 was achieved at -0.92 V versus reversible hydrogen electrode." @default.
• W2933321857 created "2019-04-11" @default.
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• W2933321857 date "2019-10-01" @default.
• W2933321857 modified "2023-10-16" @default.
• W2933321857 title "Selective electrocatalytic CO2 reduction enabled by SnO2 nanoclusters" @default.
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• W2933321857 doi "https://doi.org/10.1016/j.jechem.2018.12.004" @default.
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