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• W2936309025 abstract "Abstract Li4SiO4 is a type of very promising high-temperature CO2 sorbent, but suffers from poor cycling stability and low CO2 uptake under relatively low CO2 concentrations. In this contribution, we synthesized hierarchical Li4SiO4 nanoparticles/flakers composite from vermiculite/MCM-41 hybrid precursor and demonstrated these hybrid-type sorbents possess improved CO2 capture performance under different CO2 concentrations. The structural and morphological properties of synthesized n-(VER/MCM-41) (n = 1, 2, 3) precursors and the resulting Li4SiO4-based sorbents n-(VER/MCM-41)-Li4SiO4 were carefully characterized using XRD, SEM, BET, and XRF. Then the CO2 uptakes and CO2 sorption kinetics of n-(VER/MCM-41)-Li4SiO4 were evaluated at different temperatures (500–650 °C). We also found that the n-(VER/MCM-41)-Li4SiO4 is much less affected by CO2 concentration. Finally, the regenerative property and thermal stability of n-(VER/MCM-41)-Li4SiO4, VER-Li4SiO4, and MCM-41-Li4SiO4 were compared. In all, we demonstrated this new Li4SiO4 possesses the merits of both MCM-41-Li4SiO4 and VER-Li4SiO4 including high CO2 uptake, less effected by CO2 concentration, fast CO2 capture kinetics, and excellent cycling stability." @default.
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• W2936309025 date "2019-09-01" @default.
• W2936309025 modified "2023-10-16" @default.
• W2936309025 title "Synthesis of hierarchical Li4SiO4 nanoparticles/flakers composite from vermiculite/MCM-41 hybrid with improved CO2 capture performance under different CO2 concentrations" @default.
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• W2936309025 doi "https://doi.org/10.1016/j.cej.2019.04.072" @default.
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