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- W2937010481 abstract "As one of the more promising potential photovoltaic technologies, planar perovskite solar cells (PSCs) are arousing worldwide interest for their many advantages. Now, PSCs are being developed toward the direction of high-performance and longevity. However, the defects of the polycrystalline perovskite active layer limit further improvement of the device performance. Seeking simple and efficient strategies to reduce these trap states in the perovskite active layer is highly desirable. Here, a novel nonfunctionalized fullerene C60 o-quinodimethane bisadduct [C60(QM)2] was dissolved in chlorobenzene (CB) solvent and introduced into a CH3NH3PbI3 active layer by antisolvent dripping. Results showed that the introduced C60(QM)2 could effectively reduce the trap density of the MAPbI3 active layer, facilitating carrier extraction/injection from CH3NH3PbI3 to spiro-OMeTAD. As a result, a highest PCE of 18.4% for the PSC based on CH3NH3PbI3/C60(QM)2 was obtained, which increased by 10.1% compared with 16.7% for the reference device. Meanwhile, the air stability for C60(QM)2-passivated PSCs was also improved significantly. This approach provides a direction for designing highly efficient and air stable PSCs." @default.
- W2937010481 created "2019-04-25" @default.
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- W2937010481 date "2019-04-08" @default.
- W2937010481 modified "2023-10-15" @default.
- W2937010481 title "Enhanced Electronic Quality of Perovskite via a Novel C<sub>60</sub> o-Quinodimethane Bisadducts toward Efficient and Stable Perovskite Solar Cells" @default.
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- W2937010481 doi "https://doi.org/10.1021/acssuschemeng.9b00368" @default.
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