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- W2937704013 abstract "Exploiting molecular systems to attain tunable emission characteristics out of the organic fluorophore is of great pertinence for the construction of solid-state luminescent materials owing to their fascinating applications in optoelectronics. Herein, we have designed three charge transfer (CT) molecular assemblies utilizing carbazole luminophores (9-benzoyl carbazole (BC), 9-(para-tolyl carbazole (TC), and N-(4-formylphenyl)carbazole (FC)) as donor compounds and 1,2,4,5-tetracyanobenzene (TCNB) as an acceptor building block to tailor the structure and emission properties. Unlike TC and FC, BC has a carbonyl spacer between carbazole and phenyl group, which allow more short contacts and, therefore, effect the binary crystalline self-assembly. Detail structural and spectroscopic studies revealed the formation of alternate sandwich motifs between the donors and acceptor in a cofacial fashion, which resulted in tunable molecular structure and photophysical properties. Cocrystals XII and XIII present identical emissions due to the similar molecular packing modes (DAD···DAD) and stoichiometric ratio (2:1), whereas cocrystal XI exhibits varied molecular packing features (DADA) and molar ratio (3:2) with yellow–green fluorescence. The present study demonstrates the significance of molecular design as an effective route that could fine-tune the molecular packing, stoichiometry, and luminescence characteristics, thereby bringing out efficient optical properties out of the single component via cocrystal strategy for construction of novel solid state luminescent materials." @default.
- W2937704013 created "2019-04-25" @default.
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- W2937704013 date "2019-04-09" @default.
- W2937704013 modified "2023-09-24" @default.
- W2937704013 title "Supramolecular Design of Highly Efficient Two-Component Molecular Hybrids toward Structure and Emission Properties Tailoring" @default.
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- W2937704013 doi "https://doi.org/10.1021/acs.cgd.8b01922" @default.
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