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• W2937851805 startingPage "842" @default.
• W2937851805 abstract "Abstract Very recently, we have interestingly found that the Fe(II)-activated peroxydisulfate (PDS) process can oxidize methyl phenyl sulfoxide (PMSO) to its oxygen transfer product methyl phenyl sulfone (PMSO2), suggesting the possible occurrence of a ferryl intermediate (Fe(IV)) rather than long recognized sulfate radical (SO4 −) in this process. In this work, the formation of PMSO2 was also observed when PMSO was treated by the Fe(II)/peroxymonosulfate (PMS) system over the pH range of 3–7, and the yield of PMSO2 (i.e., the molar ratio of PMSO2 formed to PMSO lost) was quantified to be approximately 100% under acidic conditions, similar to the Fe(II)/PDS system. Moreover, 18O from isotope-labeled water (H218O) was successfully incorporated into PMSO2 product when PMSO was oxidized by the Fe(II)/PDS and Fe(II)/PMS systems in H218O, likely due to the competitive oxygen exchange of Fe(IV)-oxo species with H218O. Further, Fe(IV) evolution profiles in both systems were predicted by a Fe(IV)-mediated kinetic model, and these results are in good agreement with the experimental data obtained with a stopped-flow spectrophotometer." @default.
• W2937851805 created "2019-04-25" @default.
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• W2937851805 date "2019-09-01" @default.
• W2937851805 modified "2023-10-14" @default.
• W2937851805 title "Further understanding the involvement of Fe(IV) in peroxydisulfate and peroxymonosulfate activation by Fe(II) for oxidative water treatment" @default.
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• W2937851805 doi "https://doi.org/10.1016/j.cej.2019.04.101" @default.
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