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• W2938055998 abstract "Metal-center-driven spontaneous resolution of a pair of chiral doubly interpenetrated metal–organic frameworks (MOFs), [Ni3(ptd)6]·15.5H2O (1), which was synthesized from achiral precursors [ptd = 3-(pyridin-3-yl)-1,2,4-triazine-5,6-diol], shows vertical interpenetrated 2D → 3D frameworks with 1D channels. Interestingly, proceeding with solvothermal recrystallization in methanol, 1, with a high-symmetry tetragonal I4 space group, gives another tilted interpenetrated MOF of [Ni3(ptd)6]·10H2O·3.5MeOH (2), with low-symmetry monoclinic C2 space group. Accompanied with the structure transformation, a red shift in circular dichroism (CD) spectrum and a magnetic response (weak ferromagnetic interactions in 1 to weak antiferromagnetic interactions in 2) can be observed. Strikingly, 1 and 2 feature heterogeneous catalytic activities for the Knoevenagel reaction." @default.
• W2938055998 created "2019-04-25" @default.
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• W2938055998 date "2019-04-18" @default.
• W2938055998 modified "2023-10-16" @default.
• W2938055998 title "Spontaneous Resolution and Structure Transformation of Ni^II Metal–Organic Frameworks from an Achiral Precursor" @default.
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• W2938055998 doi "https://doi.org/10.1021/acs.cgd.9b00252" @default.
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