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- W2938482894 abstract "Environment-friendly thermoelectric SnTe has recently attracted much attention as a top candidate for replacing conventional p-type PbTe. Effective strategies leading to great advancements in this material are typified by manipulation of valence bands and chemical defects, among of which MgTe- and Cu2Te-alloying are particularly successful, respectively, for valence band convergence and lattice thermal conductivity minimization. However, pristine SnTe enables a MgTe solubility of only ∼12%, which might limit the full convergence of possibly transporting bands for an electronic performance maximization. In this work, we show an approach to increase the MgTe solubility up to ∼20%, leading to an involvement of one more highly degenerated valence band Λ for charge transport in addition to existing L and Σ bands. Such a collection of many transporting valence bands enables a great improvement in electronic performance, as well as a significant enhancement in thermoelectric figure of merit with a well-reduced lattice thermal conductivity by the point defects introduced in these SnTe alloys." @default.
- W2938482894 created "2019-04-25" @default.
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- W2938482894 date "2019-06-01" @default.
- W2938482894 modified "2023-10-10" @default.
- W2938482894 title "Maximization of transporting bands for high-performance SnTe alloy thermoelectrics" @default.
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- W2938482894 doi "https://doi.org/10.1016/j.mtphys.2019.03.005" @default.
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