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- W2938506765 abstract "Abstract CO 2 reduction by combined electro- and bio-catalytic reactions is a promising technology platform for sustainable production of chemicals from CO 2 and electricity. While heterogeneous electrocatalysts can reduce CO 2 to a variety of organic compounds at relatively high reaction rates, these catalysts have limitations achieving high selectivity for any single product beyond CO. Conversely, microbial CO 2 reduction pathways proceed at high selectivity; however, the rates at bio-cathodes using direct electron supply via electricity are commonly limiting. Here we demonstrate the use of non-precious metal cathodes that produce hydrogen in situ to support microbial CO 2 reduction to C 1 and C 2 compounds. CoP, MoS 2 and NiMo cathodes perform durable hydrogen evolution under biologically relevant conditions, and the integrated system achieves coulombic efficiencies close to 100% without accumulating hydrogen. Moreover, the one-reactor hybrid platform is successfully used for efficient acetate production from electricity and CO 2 by microbes previously reported to be inactive in bioelectrochemical systems." @default.
- W2938506765 created "2019-04-25" @default.
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- W2938506765 date "2019-04-12" @default.
- W2938506765 modified "2023-10-12" @default.
- W2938506765 title "Robust and biocompatible catalysts for efficient hydrogen-driven microbial electrosynthesis" @default.
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- W2938506765 doi "https://doi.org/10.1038/s42004-019-0145-0" @default.
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