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- W2939370650 abstract "A-site-ordered quadruple perovskite CeCu 3 Cr 4 O 12 was prepared by a high-pressure, high-temperature method at 7.7 GPa and about 1670 K. Its crystal structure was investigated using synchrotron X-ray powder diffraction between 100 and 590 K. In this temperature range, it crystallizes in the parent cubic structure for A-site-ordered quadruple perovskites with space group Im -3. It exhibits a ferrimagnetic transition at T C = 333 K. Very small changes of Cu O and Cr O bond lengths were found at T C , and no changes in Ce O bond lengths. Ce O bond lengths of CeCu 3 Cr 4 O 12 (about 2.525 Å at 290 K) were very close to those of CeCu 3 Mn 4 O 12 and CeCu 3 Fe 4 O 12 suggesting the Ce 4+ oxidation state and the charge distribution as Ce 4+ Cu 2+ 3 Cr 3.5+ 4 O 12 . No intersite charge transfer or charge disproportionation transitions were found in CeCu 3 Cr 4 O 12 . • CeCu 3 Cr 4 O 12 was prepared using a high-pressure high-temperature method. • No structural phase transitions were detected between 100 and 590 K. • CeCu 3 Cr 4 O 12 shows a ferrimagnetic transition at T C = 333 K. • CeCu 3 Cr 4 O 12 is different from BiCu 3 Cr 4 O 12 , LaCu 3 Cr 4 O 12 , and YCu 3 Cr 4 O 12 ." @default.
- W2939370650 created "2019-04-25" @default.
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- W2939370650 date "2019-07-01" @default.
- W2939370650 modified "2023-09-24" @default.
- W2939370650 title "Crystal structure and magnetic properties of A-site-ordered quadruple perovskite CeCu3Cr4O12" @default.
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- W2939370650 doi "https://doi.org/10.1016/j.jallcom.2019.04.128" @default.
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