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- W2940566669 abstract "Aqueous Fenton-reversible addition–fragmentation chain transfer (RAFT) polymerization catalyzed by heterogeneous catalysts, that is, Fe(II) metal–organic framework (MOF) particles, coupled with hydrogen peroxide (H2O2) with the reaction mixture exposed to air in open vessels is reported. Reactive hydroxyl radicals are generated via a heterogeneous redox reaction between Fe(II) of the MOF particles and H2O2, which then chemically deoxygenate the reaction mixture in situ, initiating RAFT polymerization. Well-controlled polymers (Đ < 1.1) with experimental molecular weights close to theoretical values at high monomer conversions (ca. 85%) were achieved within 15 min. High “livingness” of the synthesized polymer chains was demonstrated by chain extension experiments and matrix-assisted laser desorption/ionization time-of-flight analysis. This study contributes to the growing interest in nonenzymatic deoxygenation techniques via heterogeneous catalysis for conducting radical polymerization reactions." @default.
- W2940566669 created "2019-05-03" @default.
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- W2940566669 date "2019-04-22" @default.
- W2940566669 modified "2023-10-15" @default.
- W2940566669 title "Heterogeneously Catalyzed Fenton-Reversible Addition–Fragmentation Chain Transfer Polymerization in the Presence of Air" @default.
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- W2940566669 doi "https://doi.org/10.1021/acs.macromol.9b00038" @default.
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