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- W2942022287 endingPage "3192" @default.
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- W2942022287 abstract "N-Heterocyclic carbene catalysts are used for the first time to mediate asymmetric [8 + 2] cycloadditions of enals with tropones. The kinetic [8 + 2] cis-cycloadducts can be epimerized to their trans analogues by simply using increased amounts of base and longer reaction times. Substituted tropones are also tolerated, and the cycloaddition products can be derivatized by hydrogenation or methanolysis. The main stereochemical features of the process have been rationalized by microkinetic modeling based on the results of DFT calculations." @default.
- W2942022287 created "2019-05-03" @default.
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- W2942022287 date "2019-04-23" @default.
- W2942022287 modified "2023-10-16" @default.
- W2942022287 title "Diastereodivergent Enantioselective [8 + 2] Annulation of Tropones and Enals Catalyzed by N-Heterocyclic Carbenes" @default.
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- W2942022287 doi "https://doi.org/10.1021/acs.orglett.9b00906" @default.
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