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- W2942706624 abstract "In this paper, we explored the influence of both the variation in the molecular weight (Mn = ∼400, 2000, 4000 g/mol) and the terminal groups (hydroxyl, amino, and methoxy) on the molecular dynamics of poly(propylene glycols) confined within anodic aluminum oxide membranes of different pore diameters. All confined samples revealed the presence of two glass transition temperatures related to the vitrification of two, core and interfacial, fractions of polymers. As found, the glass transition temperature of PPG adsorbed on the pore walls increases with a decrease in polymer Mn and scales with the H-bonding ability of a given material. Surprisingly, the glass transition temperature of the core macromolecules decreases with respect to the bulk sample with increasing Mn. To gain insight into the observed quite unexpected anti-correlated behavior of both Tg values, we performed the additional contact angle and surface tension measurements together with the annealing experiments. As shown, there were no differenc..." @default.
- W2942706624 created "2019-05-09" @default.
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- W2942706624 date "2019-05-01" @default.
- W2942706624 modified "2023-09-24" @default.
- W2942706624 title "The Impact of Molecular Weight on the Behavior of Poly(propylene glycol) Derivatives Confined within Alumina Templates" @default.
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- W2942706624 doi "https://doi.org/10.1021/acs.macromol.9b00209" @default.
- W2942706624 hasPublicationYear "2019" @default.
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