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- W2942840316 abstract "Abstract We studied the temperature dependent phononic response of few-layered liquid phase exfoliated WS2 nanosheets using Raman spectroscopy over a wide temperature range from 80 to 600 K. We find that the E12g (in-plane) and A1g (out-of plane) modes follow a systematic red shift with increase in temperature and exhibits weak non-linear temperature dependence in the temperature range of 350–600 K. The first-order temperature coefficients are found to be −0.0111 cm−1 K−1 and -0.0103 cm−1 K−1 for E12g and A1g modes, respectively. From our analysis which is based on a semi-quantitative model, we find that at higher temperatures the non-linear temperature dependence of E12g and A1g modes primarily originates from the an-harmonic effects of three-phonon process as a consequence of creation of S vacancies in the WS2 nanosheets. The thermal expansion contribution is mainly dominant in low temperature region." @default.
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- W2942840316 date "2019-08-01" @default.
- W2942840316 modified "2023-09-24" @default.
- W2942840316 title "Temperature dependent Raman investigations of few-layered WS2 nanosheets" @default.
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- W2942840316 doi "https://doi.org/10.1016/j.ssc.2019.04.013" @default.
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