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• W2943064561 abstract "Electrocatalytic nitrogen reduction reaction (NRR) under ambient conditions is emerging as a potential alternative to the Haber–Bosch process when cost and environmental protection are considered. Furthermore, the grand challenge on N2 activation encourages development of efficient NRR catalysts. Herein, we report the positive effect of oxygen vacancies in Ta2O5 nanorods for effective N2 reduction. Density functional theory calculations reveal that N2 can be efficiently activated at the O-vacancy site via coordination with two Ta atoms adjacent to the O-vacancy. Electrocatalytic NRR experiments verify the superior catalytic performance of O-vacancy-engineered Ta2O5 nanorods (NH3 yield, 15.9 μg h–1 mg–1cat; Faradaic efficiency, 8.9%). This work clearly demonstrates the significance of defect engineering on the NRR field." @default.
• W2943064561 created "2019-05-09" @default.
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• W2943064561 date "2019-04-29" @default.
• W2943064561 modified "2023-10-04" @default.
• W2943064561 title "Oxygen Vacancies in Ta₂O₅ Nanorods for Highly Efficient Electrocatalytic N₂ Reduction to NH₃ under Ambient Conditions" @default.
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• W2943064561 doi "https://doi.org/10.1021/acssuschemeng.9b01178" @default.
• W2943064561 hasPublicationYear "2019" @default.
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