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- W2943078682 abstract "Molybdenum disulfide (MoS2) has a wide range of applications from electronics to catalysis. While the properties of single-layer and multilayer MoS2 films are well understood, controlling the deposited MoS2 polytype remains a significant challenge. In this work, we employ chemical bath deposition, an aqueous deposition technique, to deposit large area MoS2 thin films at room temperature. Using Raman spectroscopy and x-ray photoelectron spectroscopy, we show that the deposited MoS2 polytype can be changed from semiconducting 2H MoS2 on hydrophobic -CH3 and -CO2C6F5 terminated self-assembled monolayers (SAMs) to semimetallic 1T MoS2 on hydrophilic -OH and -COOH terminated SAMs. The data suggest that the deposition of MoS2 polytypes is controlled by the substrate surface energy. High surface energy substrates stabilize 1T MoS2 films, while 2H MoS2 is deposited on lower surface energy substrates. This effect appears to be general enabling the deposition of different MoS2 polytypes on a wide range of substrates." @default.
- W2943078682 created "2019-05-09" @default.
- W2943078682 creator A5029604099 @default.
- W2943078682 creator A5087034592 @default.
- W2943078682 date "2019-05-01" @default.
- W2943078682 modified "2023-10-18" @default.
- W2943078682 title "Polytype control of MoS2 using chemical bath deposition" @default.
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- W2943078682 doi "https://doi.org/10.1063/1.5089661" @default.
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