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- W2943113437 abstract "Selective catalytic reduction of NO with methane (NO-CH4-SCR) in the presence of excess oxygen was investigated over the synthesized MnH-ZZs-n zeolite composite catalysts with FAU (as core) and BEA (as shell) topologies. XRD, SEM, and NH3-TPD technologies were employed to characterize the catalysts. It is found that the topological structure of the zeolite affected the catalytic properties and H2O/SO2 tolerances considerably. MnH-ZZs-n catalysts exhibited much higher NO-CH4-SCR activity than the physical mixture catalysts with comparable relative mass content of Y and Beta zeolites, particularly the ratio of Y and Beta at the range of 0.2–0.5 than the MnH-Beta catalysts with single topology. NH3-TPD results showed that one new type of strong acidic sites formed in H-ZZs-n and remained in MnH-ZZs-n resulted from the interaction between the Lewis and Brönsted acid sites under a particular environment. The special zeolite-zeolite structure with ion-exchanged Mn ions in the core-shell zeolite composite catalysts contributed to the novel NO-CH4-SCR properties." @default.
- W2943113437 created "2019-05-09" @default.
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- W2943113437 date "2019-04-28" @default.
- W2943113437 modified "2023-09-27" @default.
- W2943113437 title "NO-CH4-SCR Over Core-Shell MnH-Zeolite Composites" @default.
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- W2943113437 doi "https://doi.org/10.3390/app9091773" @default.
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