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• W2943382005 abstract "Abstract The synthesis of molecular‐level artificial switchable catalysts, of which activity in different chemical processes can be switched by controlling different stimuli, has provided a new paradigm to perform mechanical tasks and measurable work. In this work, to obtain highly effective and regioselective artificial switchable catalysts, a hierarchical anion‐pillared framework {(H 3 O)[Cu(CPCDC)(4,4′‐bpy)]} n ( 1 ; H 3 CPCDC=9‐(4‐carboxyphenyl)‐9 H ‐carbazole‐3,6‐dicarboxylic acid, 4,4′‐bpy=4,4′‐bipyridine), including free [H 3 O] + ions as guest molecules, was constructed. Upon dissolve–exchange–crystallization behavior, fascinating reversible structural transformations proceeded between anion framework 1 and neutral 2D stair‐stepping framework {[Cu(CPCDC)(4,4′‐bpe)]} n ( 2 ; 4,4′‐bpe=4,4′‐vinylenedipyridine). Moreover, frameworks 1 and 2 can act as heterogeneous artificial switchable catalysts to selectively promote the direct cyanation reaction of terminal alkynes and azobisisobutyronitrile. The results indicated that 1 and 2 exhibited excellent selectivity to generate vinyl isobutyronitrile skeletons or propiolonitrile frameworks, respectively, as unique products. Furthermore, indicating paper, GC‐MS, energy‐dispersive X‐ray spectroscopy, and X‐ray photoelectron spectroscopy analysis demonstrated that the reversible structural transformations endowed 1 and 2 with well‐defined platforms to stabilize the isobutyronitrile and CN sources through the different catalytic pathways." @default.
• W2943382005 created "2019-05-09" @default.
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• W2943382005 date "2019-07-08" @default.
• W2943382005 modified "2023-10-16" @default.
• W2943382005 title "Reversible Structural Transformations of Metal–Organic Frameworks as Artificial Switchable Catalysts for Dynamic Control of Selectively Cyanation Reaction" @default.
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• W2943382005 doi "https://doi.org/10.1002/chem.201901118" @default.
• W2943382005 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31044467" @default.
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