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- W2943585343 abstract "Solar thermochemical hydrogen production has a great significance in the clean energy economy. Herein, for the first time, the direct reforming reaction of methanol into hydrogen using sunlight as the solar energy input in a homemade experiment setup is reported. Solar energy provides the thermal energy necessary for liquid evaporation and methanol reforming reaction simultaneously with the aid of the strong photo-thermal conversion property of nano-catalysts. The capillary force of sponge is utilized to promote the infiltration of nano-catalysts with the water/methanol mixture. Experimental results demonstrate that the solar-driven methanol reforming reaction takes place at a relatively low temperature (≈136 °C), and three factors, including the nano-catalyst wetting time, the molar ratio of water/methanol, as well as the solar intensity, have noticeable influence on the reaction temperature, which determines the rate of hydrogen production. The maximum solar-thermochemical conversion efficiency and solar energy utilization efficiency at optimum conditions reach 43.4% and 55.1%, respectively. The work will open a new approach for solar thermochemical energy conversion in the future." @default.
- W2943585343 created "2019-05-09" @default.
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- W2943585343 date "2019-05-15" @default.
- W2943585343 modified "2023-10-18" @default.
- W2943585343 title "A Direct Solar Photo‐Thermal Conversion of Methanol into Hydrogen" @default.
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- W2943585343 doi "https://doi.org/10.1002/ente.201900299" @default.
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