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• W2944241191 startingPage "3644" @default.
• W2944241191 abstract "A highly efficient enantio- and diastereoselective catalyzed asymmetric transfer hydrogenation via dynamic kinetic resolution (DKR-ATH) of α,β-dehydro-α-acetamido and α-acetamido benzocyclic ketones to ent- trans-β-amido alcohols is disclosed employing a new ansa-Ru(II) complex of an enantiomerically pure syn- N, N-ligand, i.e. ent- syn-ULTAM-(CH2)3Ph. DFT calculations of the transition state structures revealed an atypical two-pronged substrate attractive stabilization engaging the commonly encountered CH/π electrostatic interaction and a new additional O═S═O···HNAc H-bond hence favoring the trans-configured products." @default.
• W2944241191 created "2019-05-16" @default.
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• W2944241191 date "2019-05-06" @default.
• W2944241191 modified "2023-10-16" @default.
• W2944241191 title "<i>trans</i>-Diastereoselective Ru(II)-Catalyzed Asymmetric Transfer Hydrogenation of α-Acetamido Benzocyclic Ketones via Dynamic Kinetic Resolution" @default.
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• W2944241191 doi "https://doi.org/10.1021/acs.orglett.9b01069" @default.
• W2944241191 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6750876" @default.
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