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• W2944320802 startingPage "19066" @default.
• W2944320802 abstract "The acidity/alkalinity and structural properties of NiMgAl trimetallic oxides (MMOs) can be effectively modulated by the alkaline-etching process with various etching times, which are further used as a support to prepare KMoS-based catalysts through the cetyltrimethylammonium bromide-encapsulated Mo-precursor strategy. The enriched surface anion groups in alkaline-etched MMO affect the textural properties, metal-support interaction, and sulfidation degree of the as-synthesized KMoS-based catalysts. As a result, KMoS-based catalysts using alkaline-etched MMO as supports effectively enhance the reducibility and dispersion of Mo species, which exert a positive influence on higher alcohol synthesis (HAS) performance in CO hydrogenation. A proper balance between acidity/alkalinity and structural properties in K, Mo/MMO-x catalysts can significantly enhance the alcohol selectivity in HAS from 55 to 65% (carbon selectivity). The formation of C2+ alcohols can be boosted by adol condensation with optimal acidic/basic properties via suppressing the acidity and increasing the amount of basic sites. The alkaline-etching process also significantly improves the space time yield of C2+ alcohols over unit mass of molybdenum." @default.
• W2944320802 created "2019-05-16" @default.
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• W2944320802 date "2019-05-08" @default.
• W2944320802 modified "2023-10-13" @default.
• W2944320802 title "Alkaline-Etched NiMgAl Trimetallic Oxide-Supported KMoS-Based Catalysts for Boosting Higher Alcohol Selectivity in CO Hydrogenation" @default.
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• W2944320802 doi "https://doi.org/10.1021/acsami.9b01267" @default.
• W2944320802 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31066261" @default.
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