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- W2945015655 abstract "Experiments with the negatively charged nitrogen vacancy (N$V^-$) in diamond highlight this defect's promise for coherent storage of quantum information. They have also spurred investigations of other color centers in diamond formed by defects that consist of Group IV element (Si, Ge, Sn, Pb) and vacancies which have different atomic structure than the N$V^-$ center. To date, these other color centers have not exhibited coherence quite as impressive as that of the N$V^-$ center. Spectral diffusion and the low Debye-Waller factor are important limitations of the N$V^-$ center that make investigation of the other color centers necessary to advance the field. In this work we use density-functional theory (DFT) to study the thermodynamics and kinetics associated with the N$V$, Si$V$, Ge$V$, Sn$V$ and Pb$V$ color centers in diamond. We find agreement between our theoretical calculations and the charge state of various color centers as observed in intrinsic diamond. We determine the Fermi level values that enhance the production of isolated color centers, which may lead to longer coherence times than their present values." @default.
- W2945015655 created "2019-05-29" @default.
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- W2945015655 date "2019-05-26" @default.
- W2945015655 modified "2023-09-27" @default.
- W2945015655 title "Optimizing the Production of Single Color Centers in Diamond" @default.
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