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• W2945256433 startingPage "3602" @default.
• W2945256433 abstract "Abstract Lithium–sulfur batteries are more promising and attractive than lithium‐ion batteries owing to a higher charge‐storage capacity. However, their commercial applications are hindered by an undesirable polysulfide shuttling effect during the cycling procedure. Herein, nitrogen and sulfur codoped carbon nanotubes intertwined with flower‐like molybdenum disulfide (NSCNTs/MoS 2 ) were synthesized by using a feasible hydrothermal method and used as effective lithium polysulfides (LiPSs) tamers. The NSCNTs/MoS 2 had a strong hybrid structure with strong interfacial interactions for physical confinement, chemical adsorption, and electrocatalytic conversion of intermediate LiPSs during the charge–discharge process. The NSCNTs intensified the flexibility and constructed a conductive framework for rapid ion/electron transfer, whereas the electrocatalysis of MoS 2 managed the sulfur reaction chemistry in two ways: it chemically immobilized LiPSs through Li−S bonds and kinetically sped up the sulfur redox reactions. Owing to these merits, the Li–S cell with a NSCNTs/MoS 2 host and NSCNTs/MoS 2 ‐coated separator (NSCNTs/MoS 2 /S‐NM) exhibited a high reversible capacity of 814 mAh g −1 at 1.0 C and long‐lasting cycling durability with an ultralow capacity decay of 0.02 % per cycle over 1000 cycles. Accordingly, rationally integrating the concepts of physical immobilization, chemical capture, and electrocatalysis to establish a multifaced cell structure for the architecture of high‐performance Li–S batteries is a significant strategy." @default.
• W2945256433 created "2019-05-29" @default.
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• W2945256433 date "2019-06-27" @default.
• W2945256433 modified "2023-10-15" @default.
• W2945256433 title "Rational Fabrication of Nitrogen and Sulfur Codoped Carbon Nanotubes/MoS₂ for High‐Performance Lithium–Sulfur Batteries" @default.
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• W2945256433 doi "https://doi.org/10.1002/cssc.201900929" @default.
• W2945256433 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/31081248" @default.
• W2945256433 hasPublicationYear "2019" @default.
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