Matches in SemOpenAlex for { <https://semopenalex.org/work/W2945385004> ?p ?o ?g. }
- W2945385004 abstract "Abstract In designing the polynitrogen and nitrogen‐rich high‐energy‐density materials (HEDMs), one continuously challenged issue is to solve the severe conflict between “stability and detonation.” Most known nitrogen‐containing and nonsaltlike HEDMs involve the normally bonded skeletal nitrogens. Here, we computationally proposed a nontraditional class of nitrogen‐rich compounds with structurally uneasy nitrogens, that is, 1,3‐disubstituted cyclotetrazenes N 4 R 2 ( I ), which bear the moderate 6π‐aromaticity and slight singlet diradical character. The target N 4 R 2 ( I ) can preferably balance the “stability and detonation” necessity of HEDM, and can be fabricated into diversified compounds ranging from simple to nano‐sized high‐energy porous frameworks. The robustness of N 4 R 2 ( I ) should much expand our perceiving limitation in the nitrogen‐rich HEDM chemistry." @default.
- W2945385004 created "2019-05-29" @default.
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- W2945385004 date "2019-05-21" @default.
- W2945385004 modified "2023-10-15" @default.
- W2945385004 title "Structurally uneasy but kinetically stable nitrogens in 1,3‐disubstituted cyclotetrazenes: Viable high‐energy‐density materials" @default.
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- W2945385004 doi "https://doi.org/10.1002/qua.25976" @default.
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