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- W2945841613 abstract "Clay nanosheets (CNSs) have been widely used in the design of nanocomposite biomaterials. CNSs display a disk-like morphology with strong negatively charged surfaces. It has been shown that guanidinium-containing molecules can bind CNSs through noncovalent salt–bridge interactions and thus serve as “molecular glues” for CNSs. Making use of the guanidinium side chain in arginine, here, we designed novel arginine-rich elastomeric proteins to engineer protein-CNS nanocomposite hydrogels. Our results showed that these arginine-rich proteins can interact with CNSs effectively and can cross-link CNSs into hydrogels. Rheological measurements showed that mechanical properties of the resultant hydrogels depended on the arginine content in the arginine-rich proteins as well as CNS/protein concentration. Compared with hydrogels constructed from CNSs or proteins alone, the novel protein-CNS nanocomposite hydrogels show much improved mechanical properties. Our work opens up a new avenue to engineer functional protein hydrogels for various applications." @default.
- W2945841613 created "2019-05-29" @default.
- W2945841613 creator A5030144808 @default.
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- W2945841613 date "2019-05-13" @default.
- W2945841613 modified "2023-09-25" @default.
- W2945841613 title "Engineering Protein-Clay Nanosheets Composite Hydrogels with Designed Arginine-Rich Proteins" @default.
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- W2945841613 doi "https://doi.org/10.1021/acs.langmuir.9b00701" @default.
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