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- W2946004306 abstract "Abstract We report a comprehensive Raman scattering study on layered M PS 3 ( M =Mn, Fe, Ni), a two-dimensional magnetic compound with weak van der Waals interlayer coupling. The observed Raman phonon modes have been well assigned by the combination of first-principles calculations and the polarization-resolved spectra. Careful symmetry analysis on the angle-dependent spectra demonstrates that the crystal symmetry is strictly described by C 2h but can be simplified to D 3d with good accuracy. Interestingly, the three compounds share exactly the same lattice structure but show distinct magnetic structures. This provides us with a unique opportunity to study the effect of different magnetic orders on lattice dynamics in M PS 3 . Our results reveal that the in-plane Néel antiferromagnetic (AF) order in MnPS 3 favors a spin–phonon coupling compared to the in-plane zig-zag AF in NiPS 3 and FePS 3 . We have discussed the mechanism in terms of the folding of magnetic Brillouin zones. Our results provide insights into the relation between lattice dynamics and magnetism in the layered M P X 3 ( M =transition metal, X =S, Se) family and shed light on the magnetism of monolayer M P X 3 materials." @default.
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- W2946004306 date "2019-05-01" @default.
- W2946004306 modified "2023-10-06" @default.
- W2946004306 title "Raman scattering study of magnetic layered MPS3 crystals (${boldsymbol{M}}={rm{Mn}}$, Fe, Ni)" @default.
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- W2946004306 doi "https://doi.org/10.1088/1674-1056/28/5/056301" @default.
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