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- W2946548802 abstract "Abstract The increasing demands for the clean energy have steered the rapid development of energy storage devices with high energy and power density as well as high energy utilization efficiency. Lithium (Li)-based batteries are the most potential ones and are being intensively studied owing to their ultrahigh theoretical energy density. Despite the necessary device components including the cathodes, electrolytes and anodes, the use of interlayers is also of great significance for better performance of the battery. In lithium-sulfur (Li-S) batteries, the interlayers enable selective control of polysulfides shuttling, while not disturbing the ion transfer. In-situ formed interlayers (solid electrolyte interphase) or artificial interlayers can also modify the physico-chemical properties or prevent the formation of Li dendrites to stabilize the metallic Li anodes. Interlayers are inert in these devices but they are indispensable to construct a better operation environment for these devices just like what the cell membrane does. In this review, we discuss the most recent applications of emerging interlayer system in Li-based batteries (Li-S batteries and Li metal anode) by proposing the “cell membrane” concept as a model. We aim to use such an analogy to build up a common concept and designing principle of the interlayers for better understanding their work mechanism and fully address the significance of interlayers. This review concludes with some personal perspectives which will shed some light on the emerging requirements of the “cell-membrane-like” interlayer system for guiding future development of advanced Li-based batteries." @default.
- W2946548802 created "2019-05-29" @default.
- W2946548802 creator A5000187214 @default.
- W2946548802 creator A5005205253 @default.
- W2946548802 creator A5019017598 @default.
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- W2946548802 creator A5048448989 @default.
- W2946548802 creator A5055207576 @default.
- W2946548802 creator A5070150715 @default.
- W2946548802 date "2019-12-01" @default.
- W2946548802 modified "2023-10-16" @default.
- W2946548802 title "Interlayers for lithium-based batteries" @default.
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