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• W2947200870 abstract "Allochromatium (Alc.) vinosum has a double-peak structure of its absorption band around 800~nm. Previously, the excitonic origin of this feature has been demonstrated experimentally, but a detailed understanding still lacks a model Hamiltonian being able to reproduce absorption as well as exciton relaxation time scales. Here, we propose a system-bath model which accommodates these observables. It combines Frenkel exciton theory for a dimerized and energetically heterogeneous B800 pigment pool with a quantum master equation approach describing phase and energy relaxation according to an experimental spectral density. The analysis of this model shows that the LH2 of Alc. vinosum features an interesting interplay of two excitonic bands, which are originating from the different pigment pools." @default.
• W2947200870 created "2019-06-07" @default.
• W2947200870 creator A5025899821 @default.
• W2947200870 creator A5073567557 @default.
• W2947200870 date "2019-11-01" @default.
• W2947200870 modified "2023-09-24" @default.
• W2947200870 title "The light-harvesting complex 2 of Allochromatium vinosum: B800 absorption band splitting and exciton relaxation" @default.
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• W2947200870 doi "https://doi.org/10.1016/j.chemphys.2019.110476" @default.
• W2947200870 hasPublicationYear "2019" @default.
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