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• W2947331397 abstract "Photochromic and photoswitchable magnetic (photomagnetic) properties of spin-crossover (SCO) metal complexes in the solid state were observed almost at cryogenic temperature. Here we present a new crystalline complex [FeII(TMPT)6](ClO4)8 (TMPT = 1-(1,2,4-triazol-4-yl)-2,4,6-trimethyl-pyridinium) showing photochromism and reversible hysteresis shift, with one direction being triggered by thermal annealing and the other by irradiation at room temperature. IR/Raman and single-crystal X-ray diffraction data revealed that these behaviors are very probably induced by thermal disorder of ClO4– anions, which change intermolecular interactions and the ligand field strength of the FeII center. This discovery may inspire the design and synthesis of new photochromic and photomagnetic compounds through controlling structural disorder." @default.
• W2947331397 created "2019-06-07" @default.
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• W2947331397 date "2019-05-28" @default.
• W2947331397 modified "2023-10-14" @default.
• W2947331397 title "Photochromism and Photomagnetism Induced by Structural Disorder of a Crystalline Spin-Crossover Fe^II Complex" @default.
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• W2947331397 doi "https://doi.org/10.1021/acs.cgd.8b01885" @default.
• W2947331397 hasPublicationYear "2019" @default.
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